I struggle to think of a smoother looking pick than Spillane’s — few things better than a backer perfectly jumping the route going in the other direction.
But off the top of my head, the best picks that come to mind recently are:
Erik Harris to seal the win against the colts: https://www.nfl.com/videos/raiders-first-int-of-19-is-pick-six-from-erik-harris
Daryl Worley was a terrible CB but probably the most remarkable INT ive ever seen: https://www.youtube.com/watch?v=xbEj_r3NgB0
Jeff Heath picking Mahomes : https://www.youtube.com/watch?v=53fPEJb1awo
Kwiatkoski’s one hander against Denver https://www.raiders.com/video/nick-kwiatkoski-intercepts-drew-lock-to-finalize-win-over-denver
Woodson in the Super Bowl. I was at Qualcomm and I would have bet it all at that moment that it was going to happen.